The Tierpark in Goldau is quite nice but a few hills, you can buy boxes of food and hand feed the deer! Its also nice becasue you can combine it with the train from Arth Goldau to the top of Mt. Rigi, makes a very nice day outing.
http://www.tierpark.ch/
I also like Wildnispark, all sorts of animals some very close and a grill, you can drive or take a train very clsoe to Zurich.
http://www.wildnispark.ch/